Physical and chemical characteristics and functional properties of carbon nitride materials obtained by template synthesis

N. D. Shcherban; D. Yu. Murzin

doi:10.1007/s11237-020-09631-9

Physical and chemical characteristics and functional properties of carbon nitride materials obtained by template synthesis

N. D. Shcherban^*, D. Yu. Murzin

^*Corresponding author for this work

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Abstract

The preparation, structure, and functional properties of carbon nitride such as its photocatalytic, catalytic, and adsorption activities have been examined. The template synthesis of g-C₃N₄ allows increasing its dispersion, specific surface area, and spatial ordering, leading to enhanced photocatalytic activity of such materials in the photoreduction of carbon dioxide and larger catalytic activity in the Knoevenagel condensation as well as in the oxidation of betulin (as a support for nanodispersed ruthenium) compared with the bulk analog. Increased adsorption capacity for H₂ and CO₂ is found in the case of non-stoichiometric carbon nitride.

Original language	English
Pages (from-to)	392-397
Number of pages	6
Journal	Theoretical and Experimental Chemistry
Volume	55
Issue number	6
DOIs	https://doi.org/10.1007/s11237-020-09631-9
Publication status	Published - 26 Feb 2020
MoE publication type	A1 Journal article-refereed

Keywords

betulin oxidation
carbon dioxide photoreduction
carbon nitride
CO adsorption
Knoevenagel condensation
template synthesis

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10.1007/s11237-020-09631-9

Physical and chemical characteristics and functional properties of carbon nitride materials obtained by template synthesisAccepted author manuscript, 1.09 MBLicence: Publisher rights policy

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title = "Physical and chemical characteristics and functional properties of carbon nitride materials obtained by template synthesis",

abstract = "The preparation, structure, and functional properties of carbon nitride such as its photocatalytic, catalytic, and adsorption activities have been examined. The template synthesis of g-C3N4 allows increasing its dispersion, specific surface area, and spatial ordering, leading to enhanced photocatalytic activity of such materials in the photoreduction of carbon dioxide and larger catalytic activity in the Knoevenagel condensation as well as in the oxidation of betulin (as a support for nanodispersed ruthenium) compared with the bulk analog. Increased adsorption capacity for H2 and CO2 is found in the case of non-stoichiometric carbon nitride.",

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AU - Shcherban, N. D.

AU - Murzin, D. Yu.

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N2 - The preparation, structure, and functional properties of carbon nitride such as its photocatalytic, catalytic, and adsorption activities have been examined. The template synthesis of g-C3N4 allows increasing its dispersion, specific surface area, and spatial ordering, leading to enhanced photocatalytic activity of such materials in the photoreduction of carbon dioxide and larger catalytic activity in the Knoevenagel condensation as well as in the oxidation of betulin (as a support for nanodispersed ruthenium) compared with the bulk analog. Increased adsorption capacity for H2 and CO2 is found in the case of non-stoichiometric carbon nitride.

AB - The preparation, structure, and functional properties of carbon nitride such as its photocatalytic, catalytic, and adsorption activities have been examined. The template synthesis of g-C3N4 allows increasing its dispersion, specific surface area, and spatial ordering, leading to enhanced photocatalytic activity of such materials in the photoreduction of carbon dioxide and larger catalytic activity in the Knoevenagel condensation as well as in the oxidation of betulin (as a support for nanodispersed ruthenium) compared with the bulk analog. Increased adsorption capacity for H2 and CO2 is found in the case of non-stoichiometric carbon nitride.

KW - betulin oxidation

KW - carbon dioxide photoreduction

KW - carbon nitride

KW - CO adsorption

KW - Knoevenagel condensation

KW - template synthesis

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JO - Theoretical and Experimental Chemistry

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Physical and chemical characteristics and functional properties of carbon nitride materials obtained by template synthesis

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